Evaluation on transmutation of minor actinides discharged from PWR spent fuel in the RSG-GAS research reactor

Authors

DOI:

https://doi.org/10.11113/mjfas.v15n4.1286

Keywords:

Transmutation, minor actinide, RSG-GAS research reactor

Abstract

The evaluation of RSG-GAS research reactor for transmutation reactor was proposed to study its effectiveness to transmute minor actinides (MA), specifically Am-241, to support geologic storage/disposal. The Am-241 radionuclide was assumed to be discharged from 1000MWe PWR’s spent fuel. The mass of Am-241 discharged from within a year operation of 1000MWe PWR was 1.65E+03 gram, while the optimum Am-241 mass which can be transmuted in RSG-GAS - and still meet the safety requirements of reactivity - was 8.0E+03 gram. This was equivalent to about cumulative Am-241 discharged from 5 units of 1000MWe PWR. In 10 cycles of RSG-GAS operation (about 2 years), the remaining of Am-241 is only about 100 grams. The ratio of Am-241 transmuted (8.0E+03 gram) and Am-241 produced in the RSG-GAS core (1.98E-02 gram) within 1-year operation shows the effectiveness of RSG-GAS as a transmutation reactor.

Author Biography

Muhammad Budi Setiawan, Indonesia National Nuclear Energy Agency (BATAN)

Researcher

References

Ando, Y., and Takano, H. (1999). Estimation of LWR spent fuel composition (Report No. JAERI-RESEARCH No. 99-004). Japan Atomic Energy Research Institute, Tokyo, Japan.

Salvatores, M., and Palmiotti, G. (2011). Radioactive waste partitioning and transmutation within advanced fuel cycles: Achievements and challenges. Progress in Particle and Nuclear Physics, 66(1), 144-166.

Veliscek-Carolan, J. (2016). Separation of actinides from spent nuclear fuel: A review. Journal of Hazardous Materials 318, 266-281.

Ferhat, A., and Kitamoto, A. (1996). Concept on coupled spectrum B/T (burning and/or transmutation) reactor for treatment of minor actinides by thermal and fast neutrons. Annals of Nuclear Energy, 23(15), 1239-1248.

Setiawan, M. B., Kitamoto, A., Taniguchi, A. (2001). Evaluation on transmutation performance of minor actinides with high-flux BWR. Annals of Nuclear Energy, 28(5), 443-456.

Kitamoto, A., M. B. Setiawan, M. B., and Taniguchi, A. (2000). Progress in Nuclear Energy 37(1-4), 387-392.

Wigeland, R. A., Bauer, T. H., Hill, R. N., Stillman, J. A. (2007). Impact on geologic repository usage from limited actinide recycle in pressurized light water reactors. Journal of Nuclear Science and Technology, 44(3), 415-422.

Hussain, M., and Sohail, M. Feasibility study of transmutation of minor actinides in PWR fuel assembly. Proceeding of the 2016 International Conference on Emerging Technologies (ICET 2016). October, 18-19, 2016. Islamabad, Pakistan.

Liu, K., Wu, H., Cao, L., Zheng, Y. (2013). Studies on LLFP transmutation in a pressurized water reactor. Journal of Nuclear Science and Technology 50(6), 581-598.

Hu, W., Liu, B., Ouyang, X., Tu, J., Liu, F., …Meng, H. (2015). Minor actinide transmutation on PWR burnable poison rods. Annals of Nuclear Energy, 77, 74-82.

Liu, B., Wang, K., Tu, J., Liu, F., Huang, L., Hu, W. (2014). Transmutation of minor actinides in the pressurized water reactors. Annals of Nuclear Energy 64, 86-92.

Liu, B., Jia, R., Han, R., Lyu, X., Han, J., Li, W. (2018). Minor actinide transmutation characteristics in AP1000. Annals of Nuclear Energy 115, 116-125.

Yu, C., Li., X., Cai, X., Zou, C., Ma, Y., Han, Chen, J. (2015). Analysis of minor actinides transmutation for a Molten Salt Fast Reactor. Annals of Nuclear Energy, 85, 597-604.

Takeda, T. (2016). Minor actinides transmutation performance in a fast reactor. Annals of Nuclear Energy, 95, 48-53.

Varaine, F., Buiron, L., Boucher, L., Verrier, D., Massara, S. (2010). Study of minor actinide transmutation in sodium fast reactor depleted uranium radial blanket, Proceeding of the tenth information exchange meeting on actinide and fission product partitioning and transmutation. October, 8-10, 2008. Mito, Japan.

Mansani, L., Artioli, C., Schikorr, M., Rimpault, G., Angulo, C., de Bruyn, D. (2012). Nuclear Technology 180(2), 241-263.

Übeyli, M. (2004). Transmutation of minor actinides discharged from LMFBR spent fuel in a high power density fusion reactor. Energy Conversion and Management, 45(20), 3219-3238.

Şahin, S., Khan, M. J., Ahmed, R. (2011). Fissile fuel breeding and minor actinide transmutation in the life engine. Fusion Engineering and Design, 86(2-3), 227-237.

Setiawan, M. B., Kuntjoro, S. (2018). Preliminary analysis of high-flux RSG-GAS to transmute Am-241 of PWR's spent fuel in Asian region. Journal of Physics: Conference Series. Vol. 962. No. 1. IOP Publishing.

Surbakti, T. and Purwadi, P. (2017). Karakteristik reaktivitas teras kerja RSG-GAS selama 30 tahun beroperasi. Jurnal Penelitian Fisika dan Aplikasinya, 7(1), 13-26(14).

Downloads

Published

25-08-2019